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Radioactive sources are used for logging formation parameters. Radioactive tracers, along with the other substances in hydraulic-fracturing fluid, are sometimes used to determine the injection profile and location of fractures created by hydraulic fracturing.
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Radiotracers and markers
The oil and gas industry in general uses unsealed radioactive solids (powder and granular forms), liquids and gases to investigate or trace the movement of materials. The most common use of these radiotracers is at the well head for the measurement of flow rate for various purposes. A 1995 study found that radioactive tracers were used in over 15% of stimulated oil and gas wells.
Use of these radioactive tracers is strictly controlled. It is recommended that the radiotracer is chosen to have readily detectable radiation, appropriate chemical properties, and a half life and toxicity level that will minimize initial and residual contamination. Operators are to ensure that licensed material will be used, transported, stored, and disposed of in such a way that members of the public will not receive more than 1 mSv (100 mrem) in one year, and the dose in any unrestricted area will not exceed 0.02 mSv (2 mrem) in any one hour. They are required to secure stored licensed material from access, removal, or use by unauthorized personnel and control and maintain constant surveillance of licensed material when in use and not in storage. Federal and state nuclear regulatory agencies keep records of the radionuclides used.
As of 2003 the isotopes Antimony-124, argon-41, cobalt-60, iodine-131, iridium-192, lanthanum-140, manganese-56, scandium-46, sodium-24, silver-110m, technetium-99m, and xenon-133 were most commonly used by the oil and gas industry because they are easily identified and measured. Bromine-82, Carbon-14, hydrogen-3, iodine-125 are also used.
Examples of amounts used are:
In hydraulic fracturing, plastic pellets coated with Silver-110m or sand labelled with Iridium-192with may be added to a proppant when it is required to evaluate whether a fracturing process has penetrated rocks in the pay zone. Some radioactivity may by brought to the surface at the well head during testing to determine the injection profile and location of fractures. Typically this uses very small (50 kBq) Cobalt-60 sources and dilution factors are such that the activity concentrations will be very low in the topside plant and equipment.
Regulation in the US
The NRC and approved state agencies regulate the use of injected radionuclides in hydraulic fracturing in the United States.
The US EPA sets radioactivity standards for drinking water. Federal and state regulators do not require sewage treatment plants that accept gas well wastewater to test for radioactivity. In Pennsylvania, where the hydraulic fracturing drilling boom began in 2008, most drinking-water intake plants downstream from those sewage treatment plants have not tested for radioactivity since before 2006. The EPA has asked the Pennsylvania Department of Environmental Protection to require community water systems in certain locations, and centralized wastewater treatment facilities to conduct testing for radionuclides.