Wolle is a German surname meaning "wool". Notable people with the surname include:
Charles Robert Wolle (born 1935), American jurist from Iowa; federal judge on the U. S. District Court
Gertrud Wolle (1891–1952), German film actress
Muriel Sibell Wolle (1898–1977), American artist; known for paintings of mining communities
William D. Wolle (born 1928), American foreign service officer and ambassador
Robert H. Wolle, Sr. (born 1924), American environmentalist and public health pioneer