Alfred Smith may refer to:
Alfred Smith (artist) (1854–1932), French artist from Bordeaux
Alfred Smith (VC) (1861–1932), English soldier, recipient of the Victoria Cross in Sudan
Alfred Smith (Australian politician), Member of Parliament for Carpentaria, 1941–1960
Alfred Wellington Smith (1840–1907), merchant and politician in British Columbia, Canada
Alfred Smith (UK politician) (1860–1931), Member of Parliament for Sunderland, 1929–1931
Alfred C. Smith (1893–?), American lawyer and politician in the Virginia Senate
Al Smith (Alfred E. Smith, 1873–1944), American politician and governor
Alfred Victor Smith (1891–1915), English soldier, recipient of the Victoria Cross in World War I
Alfred Holland Smith (1863–1924), President of New York Central Railroad
Alfred Lee Smith (1838–1917), member of the New Zealand Legislative Council
Brenton Wood (Alfred Jesse Smith, born 1941), American singer/songwriter
Alfred James Smith (1901–1983), businessman and member of the Queensland Legislative Assembly
Alfred Leo Smith (1919-2014), Native American substance abuse counselor and religious freedom activist
Alf Smith (ice hockey) (1873–1953), Canadian ice hockey player
Alf Smith (Port Vale footballer), professional footballer who played for Port Vale, 1913–1918
Alf Smith (New Zealand footballer), New Zealand international football (soccer) player
Alf Smith (footballer, born 1880) (1880–1944), English footballer for Stoke
Alf Smith (Australian footballer) (1867–1936), Australian rules footballer
Alf Smith (Scottish footballer), Scottish footballer
Alfred A. Smith, American National Soccer Hall of Fame inductee
Alfred Smith (cricketer, born 1847) (1847–1915), English cricketer
Alfred Smith (cricketer, born 1812) (1812–1892), another English cricketer
Alfred Smith (Australian cricketer) (1908-1989), Australian cricketer